Curious, did you do load work-ups or pick a load and shoot it? There's a lot of maybes here and I'd hate to share a load openly that someone tries to plug n play... I've found grendel to be very forgive mg in accuracy dept. 1.5" groups at 100y being the worst of my load development on 3 rifles... Maybe something else is the issue? Can you give more information or detail on how you arrived at the loads you've tried?
Gas system has very little to do with accuracy, but functionality absolutely. My suggestion is to open it up, find a load that feeds well and shoots well, then adjust the gas system.
-Mac
Gas system controls the amount of gas that comes back which depending on the severity of the imbalance can usually cure any timing issues. Buffer weight then spring strength can alter when the brass starts to move out of the chamber. So if the gas system alone can't cure the timing then change buffer weight. If those combined don't fix it add a change in spring strength and those 3 combined can do anything you want lol. That procedure cured the timing problems on a 28" standard rifle length gas system lobbing 130s at 2500 fps. If it can fix that abomination (that rifle now wears the moniker "The Platypus") it can fix your issues.
The solid coppers are not known for speed or accuracy, just so you know. So don't expect those to match the accuracy or velocity of lead core match bullets of similar weight. Also they don't expand well at lower velocity. You may want to consider a different bullet. The combination of slow speed, lower bc, and higher velocity needed to mushroom can severely limit your effective range with those pills. Food for thought.
Lastly take the rifle apart and reassemble it. Make a note of any wiggle room any part that doesn't need to move has and try to eliminate it. Lapp your receiver face, bed the barrel extension, add shims to tighten gaps between upper and lower, ect... and get a good trigger. Stuff like that can make most ar15s shoot like a stud.
this will be the next thing I do. Will get it fully tuned then try to dial a load in again using 8208.